Life Time of Charge Carriers in Double Walled Carbon Nanotubes.
Ioannis Chatzakis,
Arifa Habib
( Kansas State University)
Mikhail Zamkov
( University of lllinois, Urbana )
Igor Lithvinuk,
Patrick Richard
( Kansas State University)
We investigate the nature of low-energy excitations in double
walled carbon
nanotubes, DWNT, by pumping the states using fs IR pulses. The
temporal
evolution of the population is examined by ionizing the resulting
population
with delayed fs UV pulses. The electron time of flight of the
ionized
electrons is recorded for a range of energies above $E_{F }$to
investigate
the relaxation dynamics of the charge carriers. The initial, fast
relaxation
is attributed to the internal thermalization of the electronic
system, and
is primarily driven by electron-electron (e-e) scattering
processes. After
the system returns to a Fermi-Dirac distribution it continues to
decay with
a slower rate associated with electron gas cooling
electron-phonon (e-ph)
interactions. We specifically want to see if the (e-e) scattering
in DWNT
follow a Fermi-liquid behavior, as observed in our previous study of
MWNT$^{1}$.
1. Zamkov, M.; Woody, N.; Shan, B.; Chang, Z.; Richard, P.
\textit{Phys. Rev. Lett.} \textbf{2005},
94, 056803.
This work was supported by the
Chemical Sciences, Geosciences and Biosciences Division,
Submitted to DAMOP, May 2006 in Knoxville, TN.
Office of Basic Energy Sciences,
Office of Science, U.S. Department of Energy.
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