Effect of electron correlation on high harmonic generation of helium atoms in intense laser fields
Xiaoxu Guan
( Department of Chemistry, University of Kansas)
Xiao-Min Tong
( University of Tsukuba, Japan)
Shih-I Chu
( Department of Chemistry, University of Kansas)
We present a time-dependent generalized pseudospectral (TDGPS)
approach in {\em hyperspherical coordinates} for fully {\em ab
initio} nonperturbative and high-precision treatment of
multiphoton electron-correlated dynamics of atomic systems in
intense laser fields [1]. The procedure is applied to the
investigation of high-order-harmonic generation (HHG) of
helium atoms in ultrashort laser pulses at a KrF wavelength of
248.6 nm. The 6D coupled hyperspherical-adiabatic-channel
equations are discretized and solved
efficiently and accurately by means of the TDGPS method. The
effects of electron correlation and doubly excited states on
HHG are explored in detail. A HHG peak with Fano line profile
is identified which can be attributed to a broad
resonance of doubly excited states. Comparison of the HHG
spectra of the {\em ab initio} two-electron and the single-
active-electron model calculations is also presented.
\vspace{1mm}
\noindent
[1] X. Guan, X.-M. Tong, and S. I. Chu, Phys. Rev. A (in
press).
This work was supported by the
Chemical Sciences, Geosciences and Biosciences Division,
Submitted to DAMOP, May 2006 in Knoxville, TN.
Office of Basic Energy Sciences,
Office of Science, U.S. Department of Energy.
Return to do another
abstract search of all our holdings.