Notes
Slide Show
Outline
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"I."
  • I. Bocharova
  • L. Cocke, I. Litvinyuk, A. Alnaser, C. Maharjan, D. Ray
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Outline
  •  Motivation
  •  Coulomb explosion imaging.
  •  Experiment requirements.
  •  Experimental setup.
  •  H2 and D2 experiments.
  •  N2 and O2 experiments.
  •  C2H2 experiment.
  •  Future plans.



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Motivation
  •  To study the structure and its time evolution of different gas molecules, using Coulomb explosion imaging
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Coulomb explosion imaging
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Why Coulomb explosion imaging?
  •     Direct method which allows for best time resolution : can use short pulses Þ Possible to observe molecules with fast dynamics such as D2
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Requirements
  • Laser impulse shorter than vibration period of molecule.
  • High intensity to produce highly charged states, so explosion potential can be approximated by Coulomb potential.
  • Minimize the thickness of molecular target beam, so that interaction volume is minimal.
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Experimental setup
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Looking for explosion fragments in coincidence
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Pump-probe
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Pump-probe setup
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(CR)EI – (Charge Resonance) Enhanced Ionization
  • Diatomic molecule: double well potential.
  • Picture is asymmetric in laser field.
  • R0 is an interatomic distance for neutral molecule.
  • Distance R between two centers increases.
  • At some critical distance Rc enhanced ionization occurs.
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D2 experment
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D2 KER vs Delay spectrum
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D2: theory and experiment
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H2 experiment
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N2 and O2 experiment
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KER Spectra for Oxygen
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KER Spectra for Nitrogen
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C2H2 : polyatomic molecule
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C2H2  acetylene and vinylidene channels separation
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Future plans
  • C2H2 experiment.


  • Continue experiments with N2 and O2.


  • CO2: triatomic molecule.
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